Monday, 9 October 2017

POLONIUM ORES

Listing description
Polonium (pronounced /pɵˈloʊniəm/, po-LOH-nee-əm) is a chemical element with the symbol Po and atomic number 84, discovered in 1898 by Marie Skłodowska-Curie and Pierre Curie. A rare and highly radioactive metalloid,[1] polonium is chemically similar to bismuth[2] and tellurium, and it occurs in uranium ores. Polonium has been studied for possible use in heating spacecraft. It is unstable; all isotopes of polonium are radioactive.
Detailed descrtption
Characteristics
Solid state form
Polonium is a radioactive element that exists in two metallic allotropes. The alpha form has a simple cubic crystal structure with an edge length of 335.2 picometres; the beta form is rhombohedral. The structure of polonium has been characterized by X-ray diffraction  and electron diffraction.
210Po (in common with 238Pu) has the ability to become airborne with ease: if a sample is heated in air to 55 °C (131 °F), 50% of it is vaporized in 45 hours, even though the melting point of polonium is 254 °C (489 °F) and its boiling point is 962 °C (1763 °F). More than one hypothesis exists for how polonium does this; one suggestion is that small clusters of polonium atoms are spalled off by the alpha decay.
Detection
Gamma counting
By means of radiometric methods such as gamma spectroscopy (or a method using a chemical separation followed by an activity measurement with a non-energy-dispersive counter), it is possible to measure the concentrations of radioisotopes and to distinguish one from another. In practice, background noise would be present and depending on the detector, the line width would be larger which would make it harder to identify and measure the isotope. In biological/medical work it is common to use the natural 40K present in all tissues/body fluids as a check of the equipment and as an internal standard.
Alpha counting
The best way to test for (and measure) many alpha emitters is to use alpha-particle spectroscopy as it is common to place a drop of the test solution on a metal disk which is then dried out to give a uniform coating on the disk. This is then used as the test sample. If the thickness of the layer formed on the disk is too thick then the lines of the spectrum are broadened, this is because some of the energy of the alpha particles is lost during their movement through the layer of active material. An alternative method is to use internal liquid scintillation where the sample is mixed with a scintillation cocktail. When the light emitted is then counted, some machines will record the amount of light energy per radioactive decay event.
Occurrence and production
Polonium is a very rare element in nature because of the short half-life of all its isotopes. It is found in uranium ores at about 100 micrograms per metric ton (1 part in 1010), which is approximately 0.2% of the abundance of radium. The amounts in the Earth's crust are not harmful. Polonium has been found in tobacco smoke from tobacco leaves grown with phosphate fertilizers.
Neutron capture
Synthesis by (n,γ) reaction
In 1934 an experiment showed that when natural 209Bi is bombarded with neutrons, 210Bi is created, which then decays to 210Po via β decay. The final purification is done pyrochemically followed by liquid-liquid extraction techniques. Polonium may now be made in milligram amounts in this procedure which uses high neutron fluxes found in nuclear reactors. Only about 100 grams are produced each year, practically all of it in Russia, making polonium exceedingly rare.
Proton capture
Synthesis by (p,n) and (p,2n) reactions
It has been found that the longer-lived isotopes of polonium can be formed by proton bombardment of bismuth using a cyclotron. Other more neutron rich isotopes can be formed by the irradiation of platinum with carbon nuclei.
Applications
When it is mixed or alloyed with beryllium, polonium can be a neutron source: beryllium releases a neutron upon absorption of an alpha particle that is supplied by 210Po. It has been used in this capacity as a neutron trigger or initiator for nuclear weapons. However, a license is needed to own and operate this form of neutron source. Other uses include the following.
  • Devices that eliminate static charges in textile mills and other places. However, beta particle sources are more commonly used and are less dangerous. A non-radioactive alternative is to use a high-voltage DC power supply to ionise air positively or negatively as required.
  • 210Po can be used as an atomic heat source to power radioisotope thermoelectric generators via thermoelectric materials.
  • Because of its very high toxicity, polonium can be used as a poison (see, for example, Alexander Litvinenko poisoning).
  • Polonium is also used to eliminate dust on film.
Toxicity
Overview
By mass, polonium-210 is around 250,000 times more toxic than hydrogen cyanide (the actual LD50 for 210Po is about 1 microgram for an 80 kg person (see below) compared with about 250 milligrams for hydrogen cyanide). The main hazard is its intense radioactivity (as an alpha emitter), which makes it very difficult to handle safely: one gram of Po will self-heat to a temperature of around 500 °C (932 °F). Even in microgram amounts, handling 210Po is extremely dangerous, requiring specialized equipment and strict handling procedures. Alpha particles emitted by polonium will damage organic tissue easily if polonium is ingested, inhaled, or absorbed, although they do not penetrate the epidermis and hence are not hazardous if the polonium is outside the body.
Acute effects
The median lethal dose (LD50) for acute radiation exposure is generally about 4.5 Sv. The committed effective dose equivalent 210Po is 0.51 µSv/Bq if ingested, and 2.5 µSv/Bq if inhaled. Since 210Po has an activity of 166 TBq per gram (4,500 Ci/g)[35] (1 gram produces 166×1012 decays per second), a fatal 4.5 Sv (J/kg) dose can be caused by ingesting 8.8 MBq (238 microcuries, µCi), about 50 nanograms (ng), or inhaling 1.8 MBq (48 µCi), about 10 ng. One gram of 210Po could thus in theory poison 20 million people of whom 10 million would die. The actual toxicity of 210Po is lower than these estimates, because radiation exposure that is spread out over several weeks (the biological half-life of polonium in humans is 30 to 50 days) is somewhat less damaging than an instantaneous dose. It has been estimated that a median lethal dose of 210Po is 0.015 GBq (0.4 mCi), or 0.089 micrograms, still an extremely small amount.
Long term (chronic) effects
In addition to the acute effects, radiation exposure (both internal and external) carries a long-term risk of death from cancer of 5–10% per Sv. The general population is exposed to small amounts of polonium as a radon daughter in indoor air; the isotopes 214Po and 218Po are thought to cause the majority of the estimated 15,000-22,000 lung cancer deaths in the US every year that have been attributed to indoor radon. Tobacco smoking causes additional exposure to polonium.
Regulatory exposure limits
The maximum allowable body burden for ingested 210Po is only 1.1 kBq (30 nCi), which is equivalent to a particle massing only 6.8 picograms. The maximum permissible workplace concentration of airborne 210Po is about 10 Bq/m3 (3 × 10−10 µCi/cm³). The target organs for polonium in humans are the spleen and liver. As the spleen (150 g) and the liver (1.3 to 3 kg) are much smaller than the rest of the body, if the polonium is concentrated in these vital organs, it is a greater threat to life than the dose which would be suffered (on average) by the whole body if it were spread evenly throughout the body, in the same way as caesium or tritium (as T2O).
210Po is widely used in industry, and readily available with little regulation or restriction. In the US, a tracking system run by the Nuclear Regulatory Commission will be implemented in 2007 to register purchases of more than 16 curies (590 GBq) of polonium 210 (enough to make up 5,000 lethal doses). The IAEA "is said to be considering tighter regulations... There is talk that it might tighten the polonium reporting requirement by a factor of 10, to 1.6 curies (59 GBq)."
Treatment
It has been suggested that chelation agents such as British Anti-Lewisite (dimercaprol) can be used to decontaminate humans. In one experiment, rats were given a fatal dose of 1.45 MBq/kg (8.7 ng/kg) of 210Po; all untreated rats were dead after 44 days, but 90% of the rats treated with the chelation agent HOEtTTC remained alive after 5 months.
Commercial products containing polonium
No nuclear authority has asserted that a commercial product was a likely source for the poisoning of Litvinenko. However, as Prof. Peter D. Zimmerman says, "Polonium 210 is surprisingly common. ...Polonium sources with about 10 percent of a lethal dose are readily available—even in a product sold on Amazon.com."
Potentially lethal amounts of polonium are present in anti-static brushes sold to photographers Many of the devices are available by mail order. General Electric markets a static eliminator module with 500 µCi (20 MBq), roughly 2.5 times the lethal dose of 210Po if 100%-ingested, for US$79; Staticmaster sells replacement units with the same amount (500 µCi) of 210Po for US$36. In USA, the devices with no more than 500 µCi of (sealed) 210Po per unit can be bought in any amount under a "general license" which means that a buyer need not be registered by any authorities: the general license "is effective without the filing of an application with the Commission or the issuance of a licensing document to a particular person."

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$12,900/KG OR $5,863.63/IB


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